Experimental and Numerical Investigation of the Performance of Luffa Fiber-Reinforced Natural Rubber Composites with Process Parameter Optimization using DOE

Abstract

Composite materials have gained significant attention due to their high strength-to-weight ratio and sustainability. In particular, natural fiber-reinforced composites are increasingly investigated as environmentally friendly alternatives to synthetic counterparts. This study focuses on fabricating lightweight and biodegradable luffa fiber-reinforced natural rubber (LNR) composites using compression molding, emphasizing optimizing key processing parameters—temperature, curing time, and compression pressure. Latex-form natural rubber was selected as the matrix owing to its biodegradability, low cost, and compatibility with natural fibers. In contrast, luffa fiber served as reinforcement due to its favorable mechanical properties. The Design of Experiments (DOE) approach, specifically Taguchi’s method, was employed to systematically analyze the influence of processing parameters on physical and mechanical performance. Experimental evaluation of mechanical properties was conducted according to ASTM standards. The rule of mixture was used to evaluate the mechanical properties analytically. The multiscale material modeling finite element (FEM) methods were used to assess the orthotropic properties using the representative volume element technique. Results showed that density was only marginally affected by processing conditions, with ROM and FEM generally overestimating values; however, FEM provided closer agreement to experimental data. Shore A hardness and longitudinal modulus highly depended on curing temperature and time, with optimal properties obtained at 100 °C for 15 min under 1.0 MPa pressure. Similarly, the maximum ultimate tensile strength (0.40 MPa) was achieved under the same conditions, attributed to enhanced fiber–matrix bonding and crosslinking. Statistical analysis (ANOVA) confirmed temperature as the most influential parameter, followed by pressure and curing time. Optimized processing conditions significantly improved fiber–matrix adhesion, resulting in superior mechanical performance. These findings provide reliable processing guidelines for developing high-performance, environmentally sustainable LNR composites, making them suitable for high-impact applications in defense and consumer sectors. © The Author(s), under exclusive licence to the Korean Fiber Society 2025.